MPI-FKF homepage > Keimer's department

Physics of strongly correlated electron systems

Our department uses neutron and x-ray diffraction and spectroscopy, optical spectroscopy, and Raman scattering, supported by various supplementary methods, to explore the structure and dynamics of materials with strong electron correlations. Topics of particular current interest include the interplay between spin, charge, and orbital degrees of freedom in transition metal oxides; mechanisms of unconventional superconductivity in solids; and quantum many-body physics at oxide interfaces. We strongly believe that close collaboration between experimentalists and theorists is essential for progress in this field. To facilitate this interaction, a small theory group operates within the department. We also have a strong effort in the development of new spectroscopic methods, especially spectral ellipsometry with synchrotron radiation and neutron resonance spin-echo spectroscopy. To this end, we operate experimental facilities at the ANKA synchrotron in Karlsruhe and at the FRM-II research reactor in Garching, in addition to our in-house laboratories. The recently commissioned TRISP spectrometer at the FRM-II allows the determination of the lifetimes of collective excitations in solids with unprecedented accuracy.

Our research projects

Unconventional superconductivity

The microscopic description of superconductivity in complex materials such as layered cuprates, cobaltates, or the recently discovered iron pnictides, is one of the most important challenges in current solid-state physics. Our group uses high-quality single crystals and state-of-the-art experimental methods to derive accurate spectra of spin and charge excitations in these materials. Such data are essential to motivate and test new theoretical concepts for the correlated electron systems that support unconventional superconductivity.

Low-dimensional magnetism

The discovery of high-temperature superconductivity has stimulated a tremendous upsurge of interest in the quantitative understanding of low-dimensional quantum magnets. Experiments performed in our group elucidate the magnetic structure and dynamics of one- and two-dimensional magnets and their influence on charge transport. Novel compounds synthesized by chemists at our institute are of particular importance.

Orbital physics

The exceptionally rich phase behavior observed in transition metal oxides originates in a competition between many-body states with different spin, orbital, and charge ordering patterns. Work in our group seeks to unravel the microscopic mechanisms underlying this competition. To this end, spectroscopic data on orbitally degenerate transition metal oxides obtained in our group are analyzed and interpreted in close collaboration with theorists.

Oxide heterostructures

Carefully controlled interfaces between two materials can give rise to novel physical phenomena and functionalities not exhibited by either of the constituent materials alone. Modern synthesis methods have yielded high-quality heterostructures and superlattices of oxide materials with competing quantum many-body states. In order to explore new correlation-driven interface phenomena, our group seeks to understand and manipulate the spin and orbital polarization at oxide interfaces (“orbital engineering”).
Recent highlights

Three-phase competition in underdoped YBa2Cu3O6+x

Resonant x-ray scattering experiments on highly ordered 'Ortho-II' YBa2Cu3O6.55 and Zn-substituted YBa2Cu3O6.6 revealed a three-phase competition between spin-modulated,charge-modulated, and superconducting states in underdoped cuprate superconductors.  
S. Blanco-Canosa et al., Phys. Rev. Lett., 2013

Wolfram-Prandl-Prize 2012

The leader of the neutron spectroscopy group Dr. Dmytro Inosov is this year's laureate of the Wolfram-Prandl-Prize for his outstanding work on iron-based high-temperature superconductors.  
Official announcement (in German)

A density-wave order that competes with superconductivity

Using resonant x-ray scattering we obtained the unambiguous evidence for long-range incommensurate charge-density-wave fluctuations competing with superconductivity in underdoped (Y,Nd)Ba2Cu3O6+x.  
G. Ghiringhelli et al., Science, 2012

Electron-phonon coupling in oxide superlattices

Raman spectroscopy reveals a long-range transfer of electron-phonon coupling between YBa2Cu3O7 and La2/3Ca1/3MnO3 layers in oxide superlattices.  
N. Driza et al., Nature Materials, 2012

Magnetic resonant mode in CeB6

Using inelastic neutron scattering, we have found a magnetic exciton mode in the non-superconducting heavy-fermion metal CeB6, resembling resonant magnetic excitations in unconventional superconductors.  
G. Friemel et al., Nature Communications, 2012

Emergent phenomena at oxide interfaces

A review article in Nature Materials discusses recent advances in understanding novel interface states that arise in oxide heterostructures due to the charge, spin and orbital reconstruction effects.  
H. Y. Hwang et al., Nature Materials, 2012

Magnetic resonant mode in the Rb2Fe4Se5 superconductor

A resonant magnetic excitation in the Rb-245 iron-selenide superconductor has been discovered at a wave vector, which differs from the ones characterizing magnetic resonant modes in other iron-based superconductors. 
J. T. Park et al. Phys. Rev. Lett., 2011
G. Friemel et al. Phys. Rev. B (R), 2012